PHAS Colloquia

Carriers’ Recombination and Enhanced Auger- Meitner processes in low-dimensional materials

by Prof. Ioannis Chatzakis

America/Chicago
Description

Hexagonal boron nitride (hBN) is a wide, indirect bandgap semiconductor with

significant potential for optoelectronic applications in the ultraviolet and mid-

infrared spectral ranges. More importantly, it is a promising platform for single-

photon emission (quantum light), making it a candidate for optical quantum qubits

operating at room temperature. The performance of such optoelectronic devices is

largely governed by the dynamics of photogenerated carriers. In this work, we

investigate the dynamics of photoexcited free carriers in exfoliated, 10B-enriched

(99%), hBN at room temperature using ultrafast spectroscopy. We identify three

distinct recombination mechanisms: a slow, excitation-independent process

attributed to Shockley−Read−Hall (SRH) recombination associated with lattice

defects and impurities; a bimolecular recombination mechanism that dominates at

moderate excitation densities; and Auger recombination, which becomes

significant at higher excitation densities. Notably, the Auger recombination rate

observed in hBN is considerably higher than in other nitride-based semiconductors.

This elevated rate is sufficient to reduce the internal quantum efficiency of hBN-

based devices under high charge carrier densities. The large Auger coefficient may

be attributed to charge localization induced by defects and impurities, as well as

strain-related built-in polarization fields. Finally, I will highlight how our work

informs the development of next-generation electronic and photonic devices,

paving the way for advancements in high-performance, energy-efficient

technologies.